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Abstract | Cited by

Heterodimeric capsules self-assembled from tetraurea calix[4]pyrrole and tetraurea calix[4]arene provide unique molecular containers for the organised inclusion of small polar molecules. By inserting stimuli-responsive groups (azobenzene) in the heterocapsule structure, we are able to modify the equilibrium state of the system or the exchange between different host–guest assemblies in a reversible manner.

Graphical abstract: Moving systems of polar dimeric capsules out of thermal equilibrium by light irradiation

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