Environmental pollution and resource waste resulting from chewed gum pose ecological concerns towards the world. However, traditional disposal approaches barely meet the requirements of low-carbon and sustainable development. High-value utilization of chewed gum is of great importance to the sustainability of human beings. Herein, versatile chewed gum/liquid metal (LM)-based flexible electronics were constructed by the stretch-knead-roller coating method. Due to strong interactions (e.g., hydrogen bonding and ion chelation), the LM micro/nano droplets were encapsulated in chewed gum without leakage. Chewed gum filled with the LM droplets exhibited firm adhesion to various substrates and could serve as self-healing flexible electronics and strain sensors. In addition, LM was wrapped on the gum surface by the roller coating method, and this chewed gum composite with superior conductivity (3.2 × 106 S m−1) and tuneable flexibility and rigidity could be knitted into smart fabrics with electro-thermal effect and electromagnetic interference-shielding performance. Therefore, the combination of LM and chewed gum not only addresses the trouble of waste disposal by turning it into a high-value product but also offers a ponderable solution for the practical application of LM.