The first direct evidence for stereoelectronic control in α deprotonation of iminium ions has been obtained by observation of selective abstraction of axial α protons from iminium ions derived from the trans-decalones (1) and (2).
H. E. Ferran, R. D. Roberts, J. N. Jacob and T. A. Spencer, J. Chem. Soc., Chem. Commun., 1978, 49 DOI: 10.1039/C39780000049
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