Issue 2, 2004
From the journal:

Journal of Materials Chemistry

Synthesis and non-linear optical properties of mono-pyrrolotetrathiafulvalene derived donor–π–acceptor dyads

Jacob Ask Hansen,a   Jan Becher,a   Jan Oskar Jeppesen,*a   Eric Levillain,b   Mogens Brøndsted Nielsen,*a   Bo Møller Petersen,a   Jan Conrad Petersenc  and  Yücel Şahind  

* Corresponding authors

a Department of Chemistry, University of Southern Denmark, Odense University, Campusvej 55, Odense M, Denmark
E-mail: joj@chem.sdu.dk, mbn@chem.sdu.dk
Fax: +45 6615 8780

b Groupe Systèmes Conjugués Linéaires, Ingénierie Moléculaire et Matériaux Organiques, CNRS UMR 6501, Université d'Angers, 2 Bd Lavoisier, Angers, France

c Danish Institute of Fundamental Metrology, Bldg. 307, Matematiktorvet, Kongens Lyngby, Denmark

d Department of Chemistry, Anadolu University, Eskişehir, Turkey

Abstract

The synthesis of novel donor–π–acceptor dyads based on a pyrrolo-annelated tetrathiafulvalene unit is described. The linear and non-linear optical properties of these chromophores have been investigated, together with their redox properties. For a dyad containing a p-nitrophenyl acceptor group, a significant third-order optical non-linearity is observed.

Graphical abstract: Synthesis and non-linear optical properties of mono-pyrrolotetrathiafulvalene derived donor–π–acceptor dyads

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Article information

DOI
https://doi.org/10.1039/B310733G
Article type
Paper
Submitted
04 Sep 2003
Accepted
05 Nov 2003
First published
01 Dec 2003

J. Mater. Chem., 2004,14, 179-184

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Synthesis and non-linear optical properties of mono-pyrrolotetrathiafulvalene derived donor–π–acceptor dyads

J. A. Hansen, J. Becher, J. O. Jeppesen, E. Levillain, M. B. Nielsen, B. M. Petersen, J. C. Petersen and Y. Şahin, J. Mater. Chem., 2004, 14, 179 DOI: 10.1039/B310733G

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