A self-reductive mesoporous CuOx/Fe/silicate nanocomposite as a highly active and stable catalyst for methanol reforming

Chien-Cheng Li; Yan-Wun Chen; Ran-Jin Lin; Ching-Chun Chang; Kuei-Hsien Chen; Hong-Ping Lin; Li-Chyong Chen

doi:10.1039/C1CC12613J

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A self-reductive mesoporous CuO_x/Fe/silicate nanocomposite as a highly active and stable catalyst for methanol reforming†

Chien-Cheng Li,^a Yan-Wun Chen,^b Ran-Jin Lin,^c Ching-Chun Chang,^d Kuei-Hsien Chen,^ad Hong-Ping Lin*^b and Li-Chyong Chen*^a

Author affiliations

* Corresponding authors

^a Center for Condensed Matter Sciences, National Taiwan University, Taipei 10617, Taiwan
E-mail: chenlc@ntu.edu.tw
Fax: +886 23366 5280
Tel: +886 23366 5249

^b Department of Chemistry, National Cheng Kung University, Tainan 701, Taiwan
E-mail: hplin@mail.ncku.edu.tw
Tel: +886 62757575 ext 65342

^c Sing-Fu consulting Co. Ltd., Ping-Dong 900, Taiwan

^d Institute of Atomic and Molecular Sciences, Academia Sinica, Taipei 10617, Taiwan

Abstract

A simple and convenient one-pot synthetic route to directly prepare a self-reductive mesoporous copper–iron–silicate (CuO_x–Fe–silicate)-based catalyst has been developed. The resultant catalyst is highly active and stable in methanol reforming without needing a pre-reduction procedure.

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Article information

DOI: https://doi.org/10.1039/C1CC12613J
Article type: Communication
Submitted: 04 May 2011
Accepted: 05 Jul 2011
First published: 20 Jul 2011

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Chem. Commun., 2011,47, 9414-9416

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A self-reductive mesoporous CuO_x/Fe/silicate nanocomposite as a highly active and stable catalyst for methanol reforming

C. Li, Y. Chen, R. Lin, C. Chang, K. Chen, H. Lin and L. Chen, Chem. Commun., 2011, 47, 9414 DOI: 10.1039/C1CC12613J

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Chemical Communications