Shape selective plate-form Ga2O3 with strong metal–support interaction to overlying Pd for hydrogenation of CO2 to CH3OH

Xiwen Zhou; Jin Qu; Feng Xu; Jingping Hu; John S. Foord; Ziyan Zeng; Xinlin Hong; Shik Chi Edman Tsang

doi:10.1039/C3CC38455A

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Shape selective plate-form Ga₂O₃ with strong metal–support interaction to overlying Pd for hydrogenation of CO₂ to CH₃OH†

Xiwen Zhou,^a Jin Qu,^a Feng Xu,^a Jingping Hu,^a John S. Foord,^a Ziyan Zeng,^b Xinlin Hong^b and Shik Chi Edman Tsang*^a

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* Corresponding authors

^a Wolfson Catalysis Centre, Department of Chemistry, University of Oxford, Oxford, UK
E-mail: Edman.Tsang@chem.ox.ac.uk

^b College of Chemistry and Molecular Sciences, Wuhan University, Wuhan, P. R. China

Abstract

A stronger metal–support interaction between Pd and plate-form Ga₂O₃ nanocrystals covered with the predominant 002 surface than other Ga₂O₃ surfaces is found, which gives higher methanol yield in catalytic CO₂ hydrogenation.

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Article information

DOI: https://doi.org/10.1039/C3CC38455A
Article type: Communication
Submitted: 24 Nov 2012
Accepted: 11 Jan 2013
First published: 11 Jan 2013

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Chem. Commun., 2013,49, 1747-1749

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Shape selective plate-form Ga₂O₃ with strong metal–support interaction to overlying Pd for hydrogenation of CO₂ to CH₃OH

X. Zhou, J. Qu, F. Xu, J. Hu, J. S. Foord, Z. Zeng, X. Hong and S. C. Edman Tsang, Chem. Commun., 2013, 49, 1747 DOI: 10.1039/C3CC38455A

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