The magnetic properties of the 5f5 [tris-(tri-1-pyrazolylborato)–plutonium(III)] complex have been investigated by ac susceptibility measurements, showing it to be the first plutonium single-molecule magnet; its magnetic relaxation slows down with decreasing temperature through a thermally activated mechanism followed by a quantum tunnelling regime below 5 K.
N. Magnani, E. Colineau, J.-C. Griveau, C. Apostolidis, O. Walter and R. Caciuffo, Chem. Commun., 2014, 50, 8171 DOI: 10.1039/C4CC03400G
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