Enhancing catalytic activity and stability for CO2 methanation on Ni@MOF-5 via control of active species dispersion

Wenlong Zhen; Bo Li; Gongxuan Lu; Jiantai Ma

doi:10.1039/C4CC08733J

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Enhancing catalytic activity and stability for CO₂ methanation on Ni@MOF-5 via control of active species dispersion†

Wenlong Zhen,^ab Bo Li,^ab Gongxuan Lu*^b and Jiantai Ma^a

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* Corresponding authors

^a State Key Laboratory of Applied Organic Chemistry, College of Chemistry and Chemical Engineering, Lanzhou University, Lanzhou, China
E-mail: zhenwenlong123@126.com
Tel: +86-931-4968-062

^b State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics, Chinese Academy of Science, Lanzhou 730000, China
E-mail: gxlu@lzb.ac.cn
Fax: +86-931-4968-178
Tel: +86-931-4968-178

Abstract

A novel, highly active catalyst Ni@MOF-5 showed unexpected activity at low temperature for CO₂ methanation. The characterization results indicated that Ni was uniformly and highly dispersed over MOF-5. This catalyst showed high stability and almost no deactivation in long term stability tests up to 100 h.

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Article information

DOI: https://doi.org/10.1039/C4CC08733J
Article type: Communication
Submitted: 03 Nov 2014
Accepted: 05 Dec 2014
First published: 05 Dec 2014

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Chem. Commun., 2015,51, 1728-1731

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Enhancing catalytic activity and stability for CO₂ methanation on Ni@MOF-5 via control of active species dispersion

W. Zhen, B. Li, G. Lu and J. Ma, Chem. Commun., 2015, 51, 1728 DOI: 10.1039/C4CC08733J

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