NH3 is a potential hydrogen energy carrier. Here we use alcohols as hole scavengers to investigate the nitrogen photofixation mechanisms including direct and indirect electron transfer processes. The t-butanol system exhibited the highest quantum yield of 36.1%, ascribing to the in situ-formed indirect electronic transmitter ˙CO2−.
W. Zhao, H. Xi, M. Zhang, Y. Li, J. Chen, J. Zhang and X. Zhu, Chem. Commun., 2015, 51, 4785 DOI: 10.1039/C5CC00589B
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