Rh-Catalyzed annulations of N-methoxybenzamides with ketenimines: synthesis of 3-aminoisoindolinones and 3-diarylmethyleneisoindolinones with strong aggregation induced emission properties

Xiaorong Zhou; Zhixing Peng; Hongyang Zhao; Zhiyin Zhang; Ping Lu; Yanguang Wang

doi:10.1039/C6CC05456K

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Rh-Catalyzed annulations of N-methoxybenzamides with ketenimines: synthesis of 3-aminoisoindolinones and 3-diarylmethyleneisoindolinones with strong aggregation induced emission properties†

Xiaorong Zhou,‡^a Zhixing Peng,‡^a Hongyang Zhao,^a Zhiyin Zhang,^a Ping Lu*^a and Yanguang Wang*^a

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* Corresponding authors

^a Department of Chemistry, Zhejiang University, Hangzhou 310027, P. R. China
E-mail: pinglu@zju.edu.cn, orgwyg@zju.edu.cn

Abstract

Rhodium-catalyzed C–H activation/annulation reactions of ketenimines with N-methoxybenzamides furnished 3-aminoisoindolin-1-ones and 3-(diarylmethylene)isoindolin-1-ones. The synthesized 3-(diarylmethylene)isoindolin-1-ones exhibited aggregation induced emissions in aqueous tetrahydrofuran solution and strong green-yellow emissions in solids.

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DOI: https://doi.org/10.1039/C6CC05456K
Article type: Communication
Submitted: 30 Jun 2016
Accepted: 02 Aug 2016
First published: 02 Aug 2016

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Chem. Commun., 2016,52, 10676-10679

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Rh-Catalyzed annulations of N-methoxybenzamides with ketenimines: synthesis of 3-aminoisoindolinones and 3-diarylmethyleneisoindolinones with strong aggregation induced emission properties

X. Zhou, Z. Peng, H. Zhao, Z. Zhang, P. Lu and Y. Wang, Chem. Commun., 2016, 52, 10676 DOI: 10.1039/C6CC05456K

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Chemical Communications

Rh-Catalyzed annulations of N-methoxybenzamides with ketenimines: synthesis of 3-aminoisoindolinones and 3-diarylmethyleneisoindolinones with strong aggregation induced emission properties†

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Rh-Catalyzed annulations of N-methoxybenzamides with ketenimines: synthesis of 3-aminoisoindolinones and 3-diarylmethyleneisoindolinones with strong aggregation induced emission properties

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