Fabrication and formation mechanism of Ce2O3–CeO2–CuO–MnO2/CNTs catalysts and application in low-temperature NO reduction with NH3†
Abstract
Ce2O3–CeO2–CuO–MnO2/CNTs catalysts were synthesized via a redox strategy, and presented 58–85% NO conversion at 80–180 °C. The 6% Ce2O3–CeO2–CuO–MnO2/CNTs catalyst displayed the optimal activity, which may be owing to the generation of amorphous mixed metal-oxide catalysts, and higher contents of Ce3+ and surface oxygen (Oy). The formation mechanism of the catalysts was proposed.