Issue 19, 2017
From the journal:

Catalysis Science & Technology

The role of various oxygen species in Mn-based layered double hydroxide catalysts in selective alcohol oxidation†

Yiyun Du,a   Qian Wang,a   Xiao Liang,a   Pengfei Yang,a   Yufei He, ORCID logo a   Junting Feng ORCID logo *a  and  Dianqing Li ORCID logo *a  

* Corresponding authors

a State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Box 98, 15 Bei San Huan East Road, Beijing 100029, China
E-mail: fengjt@mail.buct.edu.cn

Abstract

Precise identification of oxygen species in LDH-based catalysts was investigated for the first time for alcohol oxidation. Assisted by surface O2−, O2 molecules were activated in various oxidation states. Labile oxygen species could react with alcohol except for the O22− immobilized by unsaturated metals, while other oxygen species only transferred oxygen species as mediators.

Graphical abstract: The role of various oxygen species in Mn-based layered double hydroxide catalysts in selective alcohol oxidation

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Article information

DOI
https://doi.org/10.1039/C7CY00918F
Article type
Communication
Submitted
08 May 2017
Accepted
06 Sep 2017
First published
07 Sep 2017

Catal. Sci. Technol., 2017,7, 4361-4365

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The role of various oxygen species in Mn-based layered double hydroxide catalysts in selective alcohol oxidation

Y. Du, Q. Wang, X. Liang, P. Yang, Y. He, J. Feng and D. Li, Catal. Sci. Technol., 2017, 7, 4361 DOI: 10.1039/C7CY00918F

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