Here, we report a ligand- and reductant-free nickel-catalyzed N-vinylation of heteroaromatic amines using biorenewable p-cymene as a solvent. This unprecedented cross-coupling strategy has high functional group tolerance (halides, alkoxy, cyano, chiral motif, etc.) and proceeded via C–H bond activation.
V. G. Landge, J. Rana, M. Subaramanian and E. Balaraman, Org. Biomol. Chem., 2017, 15, 6896 DOI: 10.1039/C7OB01791J
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