Platinum/nitrogen-doped carbon/carbon cloth: a bifunctional catalyst for the electrochemical reduction and carboxylation of CO2 with excellent efficiency

Heng-Pan Yang; Qing Lin; Han-Wen Zhang; Guo-Dong Li; Liang-Dong Fan; Xiao-Yan Chai; Qian-Ling Zhang; Jian-Hong Liu; Chuan-Xin He

doi:10.1039/C8CC00969D

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Platinum/nitrogen-doped carbon/carbon cloth: a bifunctional catalyst for the electrochemical reduction and carboxylation of CO₂ with excellent efficiency†

Heng-Pan Yang,^a Qing Lin,^a Han-Wen Zhang,^a Guo-Dong Li,^a Liang-Dong Fan,

^a Xiao-Yan Chai,^a Qian-Ling Zhang,^a Jian-Hong Liu^a and Chuan-Xin He

*^a

Author affiliations

* Corresponding authors

^a Department of Chemistry, College of Chemistry and Environmental Engineering, Shenzhen University, Shenzhen, Guangdong, China
E-mail: hecx@szu.edu.cn
Tel: +86 0755-26536141

Abstract

A novel Pt-NP@NCNF@CC composite was prepared by the electrospinning technique. It is a highly efficient and binder-free catalyst for the direct reduction and carboxylation of CO₂ with halides. Formate with 91% Faradaic efficiency and 2-phenylpropionic acid with 99% yield could be obtained, respectively. Moreover, this catalyst has excellent stability and reusability.

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Article information

DOI: https://doi.org/10.1039/C8CC00969D
Article type: Communication
Submitted: 04 Feb 2018
Accepted: 05 Mar 2018
First published: 06 Mar 2018

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Chem. Commun., 2018,54, 4108-4111

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Platinum/nitrogen-doped carbon/carbon cloth: a bifunctional catalyst for the electrochemical reduction and carboxylation of CO₂ with excellent efficiency

H. Yang, Q. Lin, H. Zhang, G. Li, L. Fan, X. Chai, Q. Zhang, J. Liu and C. He, Chem. Commun., 2018, 54, 4108 DOI: 10.1039/C8CC00969D

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