Two mononuclear pseudotetrahedral cobalt(II) complexes with the formula Co(PNP)X2, where X = Cl (1) or X = SCN (2) and PNP = bis(2-(diphenylphosphaneyl)-4-methylphenyl)amine, have been synthesised. Magnetic and high-frequency/field electron paramagnetic resonance (HF-EPR) spectroscopy and ab initio calculation studies reveal that both complexes show uniaxial magnetic anisotropy.
Y. Zhai, Y. Deng and Y. Zheng, Dalton Trans., 2018, 47, 8874 DOI: 10.1039/C8DT01683F
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