The device level modulation of carrier transport in a 2D WSe2 field effect transistor via a plasma treatment†
Abstract
Tungsten diselenide (WSe2) has received significant attention because it shows the pristine ambipolar property arising from the Fermi level located near the midgap and can be converted to uni-polar form. In this study, we observe the formation of tungsten oxide (WOx) on the WSe2 surface after oxygen plasma treatment and show that the p-type WOx dopes WSe2. In our devices that underwent plasma treatment, it was interesting to find a strong correlation between the changes in the work function of WSe2 and a gold electrode, and the channel and contact resistances. The channel resistance changes very sensitively at a rate of 64 meV per dec with the increase in the WSe2 channel work function, which is close to the thermal limit; this indicates the defect-free oxidized WSe2 channel. The carrier transport in the oxidized WSe2 FET is shown to change to a high performance p-type device with greatly reduced channel and contact resistances with the increase in the plasma oxidation time.