Issue 12, 2021
From the journal:

Nanoscale Advances

Rational design of tandem catalysts using a core–shell structure approach†

Esteban Gioria, ORCID logo ab   Liseth Duarte-Correa,c   Najmeh Bashiri,ae   Walid Hetaba, ORCID logo cd   Reinhard Schomaecker ORCID logo e  and  Arne Thomas ORCID logo *a  

* Corresponding authors

a Technische Universität Berlin, Fakultät II, Institut für Chemie: Funktionsmaterialen, Sekretariat BA2, Hardenbergstraße 40, 10623 Berlin, Germany
E-mail: e.gioria@tu-berlin.de, arne.thomas@tu-berlin.de

b Institute of Research on Catalysis and Petrochemistry, INCAPE, UNL-CONICET, Santiago del Estero 2829, 3000 Santa Fe, Argentina
E-mail: egioria@fiq.unl.edu.ar

c Fritz Haber Institute of the Max Planck Society, Department of Inorganic Chemistry, Faradayweg 4-6, 14195 Berlin, Germany

d Max Planck Institute for Chemical Energy Conversion, Department of Heterogeneous Reactions, Stiftstraße 34-36, 45470 Mülheim an der Ruhr, Germany

e Technische Universität Berlin, Fakultät II, Institut für Chemie, Sekretariat TC 8 Straße des 17. Juni 124, 10623 Berlin, Germany

Abstract

A facile and rational approach to synthesize bimetallic heterogeneous tandem catalysts is presented. Using core–shell structures, it is possible to create spatially controlled ensembles of different nanoparticles and investigate coupled chemocatalytic reactions. The CO2 hydrogenation to methane and light olefins was tested, achieving a tandem process successfully.

Graphical abstract: Rational design of tandem catalysts using a core–shell structure approach

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Article information

DOI
https://doi.org/10.1039/D1NA00310K
Article type
Communication
Submitted
26 Apr 2021
Accepted
04 May 2021
First published
25 May 2021
This article is Open Access
Creative Commons BY-NC license

Nanoscale Adv., 2021,3, 3454-3459

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Rational design of tandem catalysts using a core–shell structure approach

E. Gioria, L. Duarte-Correa, N. Bashiri, W. Hetaba, R. Schomaecker and A. Thomas, Nanoscale Adv., 2021, 3, 3454 DOI: 10.1039/D1NA00310K

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