Coil–stretch-like transition of elastic sheets in extensional flows

Abstract

The conformation of a long linear polymer dissolved in fluid and exposed to an extensional flow is well-known to exhibit a “coil–stretch” transition, which for sufficiently long chains can lead to bistability. The present work reports computations indicating that an analogous “compact–stretched” transition arises in the dynamics of a thin elastic sheet. Sheets of nominally circular, square or rectangular shape are simulated in planar and biaxial flows using a finite element method for the sheet conformations and a regularized Stokeslet method for the fluid flow. If a neo-Hookean constitutive model is used for the sheet elasticity, the sheets will stretch without bound once a critical extension rate, as characterized nondimensionally by a capillary number, is exceeded. Nonlinear elasticity, represented with the Yeoh model, arrests the stretching, leading to a highly-stretched steady state once the critical capillary number is exceeded. For all shapes and in both planar and biaxial extension, a parameter regime exists in which both weakly stretched (compact) and strongly stretched states can be found, depending on initial conditions. I.e. this parameter regime displays bistability. As in the long-chain polymer case, the bistable behavior arises from the hydrodynamic interaction between distant elements of the sheet, and vanishes if these interactions are artificially screened by use of a Brinkman model for the fluid motion. While the sheets can transiently display wrinkled shapes, all final shapes in planar and biaxial extension are planar.