Two planar-like molecules, 1 and 2, were designed and characterized via the introduction of BNB or NBN bonds into the planar phenalenyl. Localized molecular orbital (LMO) analysis shows three 4c/2e bonds in the “hamburger” hetero-dimer (1–2) and four σ-bonds in the “waffle” homo-dimers (12 and 22), both of which have greater inter-layer interaction.
D. Li, F. Gao and H. Xu, New J. Chem., 2022, 46, 7836 DOI: 10.1039/D1NJ06166F
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