A metal–covalent organic framework catalyst with pincer coordination units for boosting transfer hydrogenation of quinolines with ammonia borane

Wenying Ai; Xiao Du; Yu Yang; Zelin Zheng; Lipeng Zhai; Baiwei Ma; Siwen Cui; Pengyu Li; Liwei Mi; Lingbo Qu

doi:10.1039/D2TA02284B

A metal–covalent organic framework catalyst with pincer coordination units for boosting transfer hydrogenation of quinolines with ammonia borane†

Wenying Ai,

*^a Xiao Du,^a Yu Yang,^a Zelin Zheng,^a Lipeng Zhai,

^a Baiwei Ma,^a Siwen Cui,^a Pengyu Li,^a Liwei Mi

*^a and Lingbo Qu*^b

Author affiliations

* Corresponding authors

^a Henan Key Laboratory of Functional Salt Materials, Center for Advanced Materials Research, School of Material and Chemical Engineering, Zhongyuan University of Technology, Zhengzhou 450007, PR China

^b College of Chemistry and Institute of Green Catalysis, Zhengzhou University, 100 Science Avenue, Zhengzhou, Henan Province 450001, People's Republic of China

Abstract

A crystalline 2D nickel-coordinated bis(imino)pyridine metal–covalent organic framework (Ni-bipy-COF) material is easily fabricated by incorporating nickel ions into the bis(imino)pyridine pincer COF skeleton. The Ni-bipy-COF catalyst can be applied to catalyze the transfer hydrogenation of quinolines with ammonia borane as a hydrogen source.

Journal of Materials Chemistry A

A metal–covalent organic framework catalyst with pincer coordination units for boosting transfer hydrogenation of quinolines with ammonia borane†

Abstract

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A metal–covalent organic framework catalyst with pincer coordination units for boosting transfer hydrogenation of quinolines with ammonia borane

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