Translucent perovskite photovoltaics for building integration

Abstract

Transparent photovoltaics provide diverse levels of average visible transmittance (AVT) along with concurrent light harvesting, making glass façades and windows accessible for photovoltaics. However, improvements in power conversion efficiency (PCE) and aesthetics are required to enhance commercial viability and public acceptance. This work presents the scalable fabrication of efficient micro-patterned translucent perovskite photovoltaics at optical qualities suited for building integration. Optimized laser-scribed transparent areas (25 μm) mitigate detrimental effects on electrical performance, featuring perovskite solar cells with 44% AVT and demonstrating industrial glass quality through neutral color rendering (CRI 97) and only 3% haze. Highlighting scalability, submodules yield PCEs of 9.0% at 32% AVT (4 cm² aperture area). The transfer to two-terminal perovskite–perovskite tandem solar cells exhibiting PCEs of 17.7% at 12% AVT and 11.1% at 31% AVT demonstrates the first translucent perovskite tandem photovoltaics. Lastly, the novel concept of transmittance gradients with 7% cm⁻¹ absolute change in AVT and 12.0% PCE for submodules is presented, providing a foundation for architectural individualizations.