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Abstract | Cited by

Ethyne elaboration of a (porphinato)Zn(II) (PZn) chromophoric core renders fine control over the zero-field splitting (ZFS) parameters of the lowest energy photoexcited triplet state (T1), resulting in the ability to manipulate the spin distribution and establish highly symmetrical coincident optical and magnetic principal axes.

Graphical abstract: The evolution of spin distribution in the photoexcited triplet state of ethyne-elaborated porphyrins

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