Enhanced photocatalytic activity of BiVO4 coupled with iron-based complexes for water oxidation under visible light irradiation

Xiangming Liang; Junqi Lin; Xiaohu Cao; Wanjun Sun; Junyi Yang; Baochun Ma; Yong Ding

doi:10.1039/C8CC09807G

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Enhanced photocatalytic activity of BiVO₄ coupled with iron-based complexes for water oxidation under visible light irradiation†

Xiangming Liang,^a Junqi Lin,^a Xiaohu Cao,^a Wanjun Sun,^a Junyi Yang,^a Baochun Ma*^a and Yong Ding

*^ab

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* Corresponding authors

^a State Key Laboratory of Applied Organic Chemistry, Key Laboratory of Nonferrous Metal Chemistry and Resources Utilization of Gansu Province, College of Chemistry and Chemical Engineering, Lanzhou University, Lanzhou 730000, China
E-mail: mabaochun@lzu.edu.cn, dingyong1@lzu.edu.cn

^b State Key Laboratory for Oxo Synthesis and Selective Oxidation, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China

Abstract

[Fe₂(TPA)₂(μ-O)Cl₂]²⁺ (TPA = tris(2-pyridylmethyl)amine) was investigated as a pre-catalyst, and greatly enhanced the photocatalytic water oxidation activity of BiVO₄. An extremely high oxygen yield of 99.1% and apparent quantum yield of 44.3% were obtained in the BiVO₄–NaIO₃ photocatalytic water oxidation system.

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Article information

DOI: https://doi.org/10.1039/C8CC09807G
Article type: Communication
Submitted: 11 Dec 2018
Accepted: 28 Jan 2019
First published: 28 Jan 2019

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Chem. Commun., 2019,55, 2529-2532

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Enhanced photocatalytic activity of BiVO₄ coupled with iron-based complexes for water oxidation under visible light irradiation

X. Liang, J. Lin, X. Cao, W. Sun, J. Yang, B. Ma and Y. Ding, Chem. Commun., 2019, 55, 2529 DOI: 10.1039/C8CC09807G

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Chemical Communications