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We report the synthesis of a bio-based, robust and recyclable thermoset polyester elastomer by using an inverse vulcanised sulfur-polymer (SP) as a crosslinker for a bio-based polyester elastomer (BPE). The cross-linkages inherited from SP are mainly composed of dynamic di- and poly-sulfide bonds, which endow the crosslinked BPE with superior mechanical properties and the ability to be malleable and recyclable.

Graphical abstract: A bio-based, robust and recyclable thermoset polyester elastomer by using an inverse vulcanised polysulfide as a crosslinker

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