Kaiwen
Luo
a,
Zhijing
Huang
ac,
Xianpeng
Lv
a,
Wentao
Qiu
a,
Heyuan
Guan
a,
Tiefeng
Yang
ad,
Thierry
Grosjean
*b and
Huihui
Lu
*ad
aGuangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications, Department of Optoelectronic Engineering, Jinan University, Guangzhou 510632, China. E-mail: thuihuilu@jnu.edu.cn
bCNRS, FEMTO-ST Institute UMR 6174, Université Bourgogne Franche-Comté, Besançon 25000, France. E-mail: thierry.grosjean@univ-fcomte.fr
cSchool of Electronics and Communication, Guangdong Mechanical and Electrical Polytechnic, Guangzhou 510550, China
dKey Laboratory of Optoelectronic Information and Sensing Technologies of Guangdong Higher Education Institutes, Jinan University, Guangzhou 510632, China
First published on 6th February 2023
We study the magnetic spin-locking of optical surface waves. Through an angular spectrum approach and numerical simulations, we predict that a spinning magnetic dipole develops a directional coupling of light to transverse electric (TE) polarized Bloch surface waves (BSWs). A high-index nanoparticle as a magnetic dipole and nano-coupler is placed on top of a one-dimensional photonic crystal to couple light into BSWs. Upon circularly polarized illumination, it mimics the spinning magnetic dipole. We find that the helicity of the light impinging on the nano-coupler controls the directionality of emerging BSWs. Furthermore, identical silicon strip waveguides are configured on the two sides of the nano-coupler to confine and guide the BSWs. We achieve a directional nano-routing of BSWs with circularly polarized illumination. Such a directional coupling phenomenon is proved to be solely mediated by the optical magnetic field. This offers opportunities for directional switching and polarization sorting by controlling optical flows in ultra-compact architectures and enables the investigation of the magnetic polarization properties of light.
Our research refers to the spin-momentum locking of light—an optical SOI effect associated with evanescent waves. In such waves, the elliptically polarized electric or magnetic field describes a transverse spin angular momentum whose sign flips when propagating along opposite directions. With a subwavelength (dipolar) coupler, the longitudinal spin angular momentum (SAM) of an impinging wave can be transferred into the transverse SAM of the evanescent tail of a guided mode, leading to a directional light coupling and guiding wave. This robust spin-controlled directionality has been demonstrated with various optical systems including nanofibers,18 waveguides,19–22 and surface wave modes.23–27 So far, most investigations focused on using the rotating electric component of light as the source of SAM for originating the transverse spin-direction coupling.27–29 A recent study demonstrated that the magnetic component of light can play the same role of offering SAM in the SOI of light.17 In that work, the light coupler has an electric dipole response, leading to a power conversion to the waves driven by the electric optical field. The magnetic field is only responsible for the directionality control of the Bloch surface waves (BSWs). Here, to exclude any influence from the electric field in the coupling process, we turn to use a magnetic dipole (MD) coupler which can be configured by shaping a nanoparticle and show a pure magnetic coupling of light to BSWs. BSWs are electromagnetic surface waves excited at the interface between a periodic dielectric multilayer and its surrounding medium,17 and they can be excited by both TE- and TM-polarized waves, which offers an appropriate platform for the manipulation of polarization.
High-index dielectric nanoparticles can support MD mode. Working on Mie resonance, strong volume displacement currents are induced in these nanoparticles, which promotes the effective magnetic polarizability to be comparable or even stronger than the electric polarizability.30,31 High-index dielectric nanoparticles thus provide a versatile platform for studying magnetic light–matter interactions.30,32–34 Furthermore, the spectral position and relative strength of electric and magnetic optical resonances can also be independently tailored by changing the shape35 and composition36–38 of the nanoparticle. By this approach, a directional far-field scattering has been achieved. Besides, the huge potential of high-index dielectric nanoantennas for directional excitation of surface waves and their highly efficient demultiplexing has been revealed.35
In this paper, we study the spin-locking of BSWs solely mediated by the magnetic field of light. BSWs are surface modes propagating on top of a one-dimensional photonic crystal (1D-PC). We configure the dielectric multilayers of our 1D-PC to ensure a pure TE-polarized BSW mode in which only the magnetic field spins. A Mie scatterer is used as a near-field light-to-BSW coupler and circularly polarized light is projected onto the scatterer for studying the directional excitation of BSWs. We find that the excitation directionality of BSWs can be manipulated by spin-locking the magnetic SOI of light. This demonstration offers opportunities for directional switching and polarization sorting by controlling optical flows in ultra-compact architectures and enables the analysis of the polarization properties of light.
The dipole source is assumed located in air with a vertical distance z0 from the top surface of the waveguide. Its interaction with the waveguide can be described by Fermi's Golden Rule.18,39–41 The directional excitation of the waveguide refers to the asymmetric distribution of the total coupled energy in the two counter-propagating guided waves. Such a coupling directionality originates from the interference of the respective optical excitations aroused by the two orthogonal components of the dipolar moment (dx and dz), which can be either destructive or constructive depending upon the propagation direction. In general, a properly chosen polarization of the dipole will result in destructive interference in one prescribed direction and a mode propagating in the opposite direction.16,27,42 Alternatively, this directional phenomenon can be interpreted from the dipole side by inspecting its angular spectrum.16,42
Following the angular momentum approach, a magnetic (electric) field can be resolved into a set of plane-wave and evanescent-wave components:
(1) |
(2) |
To better understand the spin-locking effect while coupling a spinning dipole (elliptically or circularly polarized) to evanescent waves, we measure the dipolar directionality factor as follows:16
(3) |
Fig. 1(b) and (c) show the angular spectra of a dipole oriented in the z- and x-directions, respectively. We can see that the angular spectrum is an odd function of kx for the vertical dipole while even for the horizontal one. The superposition of the two dipoles can therefore lead to a strongly asymmetric function of kx. By combing the two orthogonal dipoles with proper linear coefficients, the angular spectra of the dipoles with various polarization states are obtained and plotted in Fig. 1(d). The composed dipolar field varies with the polarization state of the dipole. Remarkably, in certain cases, distinct symmetries appear in the propagating and evanescent spatial components.
As shown in Fig. 1(d), the evanescent angular spectrum (|kx| > k0, where k02 = kx2 + kz2) of an elliptically or circularly polarized dipole is strongly asymmetric to kx, which is in favor of directionality in their near-field interaction with matter. The propagating components of these dipoles (|kx| < k0), however, are always symmetric disregarding the sign of kx. Such a difference means that one can expect a directional phenomenon from a spinning dipole only by presenting it in proximity to the waveguide. In this way, the evanescent fields associated with the dipole and guided mode overlap and hence crosstalk efficiently. It is noted that, by introducing nanostructures to locally break the symmetry of an optical waveguide, a directional phenomenon can also be realized with linear polarization.43 Nevertheless, when it comes to ordinary waveguides, one loses the directionality since a linear dipole contains symmetric evanescent components, as shown in Fig. 1(e) and (f).
Quantitative assessment of the coupling directionality of a dipole to a waveguide can be made following the procedures described in the literature.16,27,42 The discussion above relates only to the angular components of the dipole itself in the air as shown in Fig. 1(b–d), with no mention being made of the nearby waveguide. When a dipole is placed close to a surface, due to the conservation of transverse momentum, the probability of exciting guided modes with specific (kx, ky) is proportional to the amplitude of the corresponding spatial component in the dipolar field, weighted by the Fresnel reflection coefficients.16 Therefore, when a spinning dipole possessing a strongly asymmetric spectrum in its evanescent components is placed near a surface or planar waveguide, it develops a highly directional excitation of the guided modes.16 As can be inferred from Fig. 1(c), a unidirectionality is attainable with proper helicity of the spinning magnetic dipole. Besides, one can play with the coupling directionality by tuning the ellipticity of the magnetic dipole. Such a tunable distribution of the coupled energy is ultimately due to the SAM transfer from the dipole source to the guided mode, which must obey the conservation law of angular momentum.
So far, we have analytically shown that a spinning magnetic dipole could develop a spin-controlled excitation of optical guided modes. To verify that, we numerically investigate the coupling of circularly polarized magnetic and electric dipoles to BSWs by the finite-difference time-domain (FDTD) method with a commercial code (Lumerical FDTD Solutions). To this end, we carry out two sets of simulations with the dipole positioned 10 nm above the top surface of a 1D-PC. The material and geometry of the 1D-PC are shown in Fig. S1 of the ESI,† which is configured as those in previous literature17 so that it supports a pure TE mode at the wavelength of 1550 nm.
Fig. 2 shows the simulation results obtained by using electric and magnetic dipoles of various polarization states to excite the 1D-PC. We can see from Fig. 2 (c–f) that the BSWs excited by a spinning magnetic dipole are strongly unbalanced on the left and right sides. The preferential side is dictated by the handedness of the dipole. In addition, we can find that even if the rotating magnetic dipole is not exactly in circular polarization (1, ±i), the directionality of TE-BSWs still exists, which is aligned with the directionality predicted by the angular momentum. It is noted that, however, a spinning electric dipole polarized in the xz-plane can hardly excite the TE-BSWs, as shown in Fig. S2 of the ESI.† A linearly polarized electric dipole oriented in the y-direction can excite the BSWs but leads to a symmetric distribution on both sides. A tunable directional excitation of the BSWs here is thus solely controlled by the magnetic field of light. Indeed, for TE-polarized BSWs only the magnetic field spins and describes the transverse SAM involved in the spin-locking effects.17
From the above calculations, the directionality predicted by the angular momentum and numerical simulations matches well. Both show a tunable directionality controlled by the optical magnetic field.
In this paper, we seek a spinning magnetic dipole at the wavelength of 1550 nm. To this end, two types of nanoparticles are investigated: (i) a solid silicon sphere and (ii) a core–shell structure with gold and silicon as the materials of the core and shell, respectively. We numerically study the dependence of scattering resonances on the sizes of these nanoparticles.
Fig. 3(a) shows the scattering spectra of core–shell structures with a constant core radius of 70 nm and various shell radii ranging from 180 nm to 280 nm. As a comparison, Fig. 3(c) displays the scattering spectra of a silicon sphere whose radius is tailored within the same range. The scattering spectra of the two types of nanoparticles share some common characteristics. First, one can recognize three sources of optical resonance: the electric dipole (ED), magnetic dipole (MD), and magnetic quadrupole (MQ) resonances. The relative strength of these resonances varies with the structure size and operation wavelength. Second, the MQ resonance becomes much less significant around the wavelength of 1550 nm though it is remarkable at shorter wavelengths. Finally, in both structures the MD resonance dominates at λ = 1550 nm but for different reasons. As to the core–shell structure, this phenomenon results from the spectral overlapping of the ED and MD resonances as the radius of the silicon shell increases. For the silicon sphere, however, only the MD resonance holds at the wavelength of around 1600 nm. These differences are more clearly shown in Fig. 3(b) and (d), which plot the spectra of the scattering cross-section of the MD and ED resonances, respectively.
From the above discussion, one can see that both the silicon sphere and gold–silicon core–shell structure are good candidates for our purpose. However, it is known that the scattering and resonant properties of a dipolar source will be modified by a substrate present nearby.45–47 We numerically investigate the influences of the substrate on the optical responses of the nanoparticles. Fig. 3(e) and (f) show respectively the simulated scattering cross-section spectra of the two nanoparticles in air and with two types of substrates presented, namely a dielectric slab and the 1D-PC. As shown in Fig. 3(e), the dielectric slab redshifts the MD resonant peak of the core–shell structure to 1600 nm while the 1D-PC only causes a negligible spectral shift. A distinct influence of the substrate is found with the silicon sphere that both the dielectric slab and 1D-PC blue-shift the MD resonance by a comparable amount of 50 nm (see Fig. 3(f)).
To clearly demonstrate the quantitative relationship between the electric and magnetic responses in nanoparticles, we give the formula to calculate the ratio of the MD components:
(4) |
As shown in Fig. S3 of the ESI,† the silicon sphere shows better MD response than the core–shell structure on resonance at λ = 1550 nm. In addition, the MD resonance of the silicon sphere is also blue-shifted by 50 nm due to the influence of 1D-PC, which results in a much larger ratio of the MD than the core–shell structure. The MD-like optical response of the nanoparticles has been further confirmed by inspecting their emission patterns. In these numerical studies, we use a commercial finite-element electromagnetic solver (the RF module of COMSOL Multiphysics). The results are shown in Fig. 3(g), (h) and S4 of the ESI.† Such a doughnut shape characterizes the far field of an MD which is shown in Fig. 3(h). Indeed, if considerable amounts of ED or high-order multipole resonances were involved, the scattering pattern would lose its perfect symmetry.48 Therefore, with the optimal design of the two nanoparticles, we have found that the silicon sphere with a radius of 220 nm exhibits better MD properties than the core–shell structure at λ = 1550 nm in the presence of the 1D-PC.
The above-described scheme has been used to demonstrate the spin-locking effects associated with the electric or magnetic fields of light.17 We follow this idea and adopt a silicon sphere as the light-to-BSW coupler (see Fig. 4(a)). It is noted that the nanoparticle merely produces a symmetric field distribution under the illumination of linearly polarized incident light, as shown in Fig. 4(b).
We illuminate the nanoparticles at four incidence angles (α = 30°, 45°, 60°, and 80°) to see how the spin-locking effect comes to work. Fig. 4(c) shows the corresponding simulation results obtained with circularly polarized light of opposite handedness. The elongated spot indicated by the thicker white arrow is the cross-section of the excitation beam along the surface of the 1D-PC. The two thinner white arrows mark the emerging BSWs where one can see an unbalanced intensity distribution on the two sides. Besides, the preferential excitation toggles from one side to the other as we inverse the handedness of the incident light, revealing a spin-dependent characteristic of this phenomenon. As the incident angle increases, the intensity distribution asymmetry in the emerging BSWs becomes more and more pronounced. When α = 80°, the coupled energy is almost steered to only one side. To better visualize the asymmetry, we compute the far-field image shown in Fig. 4(d). As can be seen from the figure, no directionality is observed without nanoparticles, but obvious directionality appears after placing the silicon sphere, which demonstrates a directional BSW excitation. Moreover, Fig. 4(e) and (f) show that under the illumination of circularly polarized incident light when α = 80°, the BSWs on the side of stronger intensity are off-center by about 30°.
We see above that the coupling directionality improves as the incident angle increases. That is because the SAM of the BSWs is transverse while that of the incident photons is longitudinal regarding their respective propagation directions. A larger incident angle of the impinging light will lead to a better alignment of the two SAMs and thus a higher coupling directionality. In purely TE-polarized BSWs, only the magnetic field rotates. Therefore, the observed spin-locking directionality is solely controlled by the magnetic field of the incident light.
J′(θ) = R−1(θ) × M × R(θ) × J | (5) |
The rotation of QWP regarding the fixed LP dynamically modulates the properties of the light impinging on the nanoparticle. Its helicity has a 180°-periodicity with respect to the angle θ, which thus dictates a 2θ-dependence for any helicity-dependent optical phenomena. Besides, the electromagnetic amplitude of the incident light, when projected on the polarization vectors of BSWs, also undergoes a 2θ-modulation. Therefore, the excitation rate of BSWs has a 4θ-dependence due to their proportionality to the optical intensity. Such modulations of different periodicity are critical for identifying the origins of the magnetic spin-locking effect.17 In our numerical simulations (FDTD method), two light sources of orthogonal linear polarization are used separately to excite the nanoparticle. The obtained results are linearly combined to construct the result at an arbitrary polarization state of the incident light. The combination coefficients are identical to the elements in J′. We consider a 360°-rotation of the QWP and plot the intensity of BSWs on the left and right sides as a function of θ. The integral area of the electric field is shown in Fig. S6(a) of the ESI.† We can see that in Fig. 5 all BSW intensity curves show similar characteristics, namely a 4θ-harmonic function undergoing a 2θ-harmonic modulation. Besides, one can see from the curves a spin-dependent directionality with a 180°-periodicity. These observations are consistent with our predictions.
To better understand the 2θ- and 4θ-modulations in the recorded signals, we apply Fourier transforms to get them expressed in the following analytical form:
(6) |
As shown in Fig. 5, the intensity signals consist of harmonic functions of the zeroth, second, and fourth order. The second harmonics is associated with the energy coupling from light into BSWs resulting from the spin-controlled distribution. Moreover, due to the TE-polarized nature of our BSWs (only the magnetic field spins), such a helicity-dependent energy distribution is solely related to the magnetic field of the incident light. It is noted that since here we use a MD coupler, both the second and fourth harmonics should be attributed to magnetic effects. This is different from the literature [17] where an electric coupler was used (see Table S1 of the ESI†).
We see that in Fig. 5(b) the ratio of the second harmonic component to the fourth harmonic is higher than that in Fig. 5(d), which shows that the magnetic optical effect plays a larger role in spin-controlled coupling by using a silicon sphere. (For more details, please refer to Fig. S6(b) of the ESI†.)
Given the symmetry of our photonic platform, the optical energies transmitted in the two silicon waveguides are proportional to those coupled from the incident light to the left and right branches of BSWs. The excitation directionality of BSWs can thus be evaluated with the following directionality factor:
(7) |
Fig. 6(b) and (c) show the propagating modes excited in the silicon waveguides upon circularly polarized illumination of opposite handedness. They show a strongly unbalanced intensity distribution in the two waveguides with a directionality factor C up to 4.58 in Fig. 6(b). Besides, inversing the handedness of the incident light switches the prevailing side from one to another with a directionality factor C = 1/4.58, manifesting a spin-dependent characteristic of this phenomenon. In contrast, with linearly polarized incident light, the coupled energy is equally distributed (C = 1). According to Section 4 (the energy coupling to BSWs), changing the polarization state of the incident light allows us to tunably control the value of C, which can be utilized to build on-chip light routers.
Footnote |
† Electronic supplementary information (ESI) available. See DOI: https://doi.org/10.1039/d2na00899h |
This journal is © The Royal Society of Chemistry 2023 |