The contribution of mixed-valence electron delocalisation to the ferromagnetic exchange between the iron(III) ions in Prussian Blue {FeIII4[eII(CN)6]3·14H2O} has been estimated theoretically. Agreement between the calculated and observed values of the Curie temperature is quite good.
B. Mayoh and P. Day, J. Chem. Soc., Dalton Trans., 1976, 1483 DOI: 10.1039/DT9760001483
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