An attempt is made to choose between the concept that the radical cation of tetramethylurea is stable, and has its SOMO confined to one nitrogen, and the concept that it decomposes to give ·NMe2 radicals and Me2NCO+ cations.
M. C. R. Symons, J. Chem. Soc., Chem. Commun., 1987, 866 DOI: 10.1039/C39870000866
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