The first organocatalytic “anti-Michael” reaction of cyclic-β-ketoesters to unsaturated double bonds is described in a highly asymmetric version leading to the synthesis of α,α′-disubstituted branched double bonds as optically active Baylis–Hillman-like adducts.
J. Alemán, E. Reyes, B. Richter, J. Overgaard and K. A. Jørgensen, Chem. Commun., 2007, 3921 DOI: 10.1039/B710393J
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