Issue 37, 2011
From the journal:

Chemical Communications

Zn-containing porphyrin as a biomimetic light-harvesting molecule for biocatalyzed artificial photosynthesis†

Jae Hong Kim,a   Sahng Ha Lee,a   Joon Seok Lee,a   Minah Leea  and  Chan Beum Park*a  

* Corresponding authors

a Department of Materials Science and Engineering, Korea Advanced Institute of Science and Technology, Science Road 335, Yuseong-gu, Daejeon, Republic of Korea
E-mail: parkcb@kaist.ac.kr
Fax: +82 42 350 3310
Tel: +82 42 350 3340

Abstract

Among the porphyrin molecules with different metal insertion sites and functional ligands, Zn-porphyrin most efficiently regenerates NADH through photo-induced electron transfer in the presence of [Cp*Rh(bpy)H2O]2+, a rhodium-based electron mediator. Photochemical regeneration of NADH by Zn-porphyrin is successfully coupled with redox enzymatic synthesis under dark state conditions.

Graphical abstract: Zn-containing porphyrin as a biomimetic light-harvesting molecule for biocatalyzed artificial photosynthesis

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Article information

DOI
https://doi.org/10.1039/C1CC12222C
Article type
Communication
Submitted
18 Apr 2011
Accepted
24 Jun 2011
First published
11 Jul 2011

Chem. Commun., 2011,47, 10227-10229

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Zn-containing porphyrin as a biomimetic light-harvesting molecule for biocatalyzed artificial photosynthesis

J. H. Kim, S. H. Lee, J. S. Lee, M. Lee and C. B. Park, Chem. Commun., 2011, 47, 10227 DOI: 10.1039/C1CC12222C

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