Design of a highly ordered mesoporous H3PW12O40/ZrO2–Si(Ph)Si hybrid catalyst for methyl levulinate synthesis

Fang Su; Ling Ma; Daiyu Song; Xianghuan Zhang; Yihang Guo

doi:10.1039/C3GC36912A

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Design of a highly ordered mesoporous H₃PW₁₂O₄₀/ZrO₂–Si(Ph)Si hybrid catalyst for methyl levulinate synthesis†

Fang Su,^a Ling Ma,^a Daiyu Song,^a Xianghuan Zhang^a and Yihang Guo*^a

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* Corresponding authors

^a School of Chemistry, Northeast Normal University, Changchun, P. R. China
E-mail: guoyh@nenu.edu.cn
Tel: +86 431 85098705

Abstract

A highly ordered mesoporous ZrO₂-based material functionalized by benzene-bridged organosilica groups and the Keggin type heteropolyacid, prepared in a single co-condensation–hydrothermal treatment step, exhibited much higher catalytic activity towards methyl levulinate synthesis compared to alkyl-free H₃PW₁₂O₄₀/ZrO₂.

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Article information

DOI: https://doi.org/10.1039/C3GC36912A
Article type: Communication
Submitted: 29 Nov 2012
Accepted: 31 Jan 2013
First published: 31 Jan 2013

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Green Chem., 2013,15, 885-890

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Design of a highly ordered mesoporous H₃PW₁₂O₄₀/ZrO₂–Si(Ph)Si hybrid catalyst for methyl levulinate synthesis

F. Su, L. Ma, D. Song, X. Zhang and Y. Guo, Green Chem., 2013, 15, 885 DOI: 10.1039/C3GC36912A

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