Coherent electron spin manipulation in a dilute oriented ensemble of molecular nanomagnets: pulsed EPR on doped single crystals

Fabrizio Moro; Danielle Kaminski; Floriana Tuna; George F. S. Whitehead; Grigore A. Timco; David Collison; Richard E. P. Winpenny; Arzhang Ardavan; Eric J. L. McInnes

doi:10.1039/C3CC46326E

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Coherent electron spin manipulation in a dilute oriented ensemble of molecular nanomagnets: pulsed EPR on doped single crystals†

Fabrizio Moro,^a Danielle Kaminski,^b Floriana Tuna,^a George F. S. Whitehead,^a Grigore A. Timco,^a David Collison,^a Richard E. P. Winpenny,^a Arzhang Ardavan^b and Eric J. L. McInnes*^a

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* Corresponding authors

^a School of Chemistry and Photon Science Institute, The University of Manchester, Oxford Road, Manchester M13 9PL, UK
E-mail: eric.mcinnes@manchester.ac.uk
Fax: +44 (0)161-275-1001
Tel: +44 (0)161-275-4469

^b CAESR, The Clarendon Laboratory, Department of Physics, University of Oxford, Parks Road, Oxford OX1 3PU, UK
E-mail: a.ardavan1@physics.ox.ac.uk
Tel: +44 (0)1865 272366

Abstract

Doping a Cr₇Zn molecular nanomagnet into a diamagnetic and isostructural host allows pulsed X-band EPR on single crystals, including relaxation and nutation experiments on the S = 3/2 ground state.

This article is part of the themed collections: Celebrating our 2019 Prize and Award winners and Molecular Spintronics

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DOI: https://doi.org/10.1039/C3CC46326E
Article type: Communication
Submitted: 17 Aug 2013
Accepted: 29 Oct 2013
First published: 04 Nov 2013
This article is Open Access

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Chem. Commun., 2014,50, 91-93

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Coherent electron spin manipulation in a dilute oriented ensemble of molecular nanomagnets: pulsed EPR on doped single crystals

F. Moro, D. Kaminski, F. Tuna, G. F. S. Whitehead, G. A. Timco, D. Collison, R. E. P. Winpenny, A. Ardavan and E. J. L. McInnes, Chem. Commun., 2014, 50, 91 DOI: 10.1039/C3CC46326E

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Chemical Communications

Coherent electron spin manipulation in a dilute oriented ensemble of molecular nanomagnets: pulsed EPR on doped single crystals†

Abstract

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Coherent electron spin manipulation in a dilute oriented ensemble of molecular nanomagnets: pulsed EPR on doped single crystals

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