Polyampholyte-based films can be efficiently self-assembled onto a surface in a one-pot manner. By using a gradient of protons, morphogens, generated at an electrode surface, a charge-shifting polyelectrolyte present in solution can be transformed into a polyampholyte, leading to the continuous buildup of a film based on polyelectrolyte complexation.
T. Garnier, A. Dochter, N. T. T. Chau, P. Schaaf, L. Jierry and F. Boulmedais, Chem. Commun., 2015, 51, 14092 DOI: 10.1039/C5CC04477D
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