Modification of the classic terpyridine pincer ligand with pendent NHR (R = mesityl) groups provides enhanced activity and stability in Ru-catalyzed dehydrogenation catalysis. These second sphere modifications furnish highly active catalysts for the oxidant-free dehydrogenative oxidation of primary alcohols to carboxylates and facilitate catalyst recycling.
E. W. Dahl, T. Louis-Goff and N. K. Szymczak, Chem. Commun., 2017, 53, 2287 DOI: 10.1039/C6CC10206A
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