A non-interpenetrating lead-organic framework with large channels based on 1D tube-shaped SBUs

Fangna Dai; Weidong Fan; Xue Yuan; Zhaodi Huang; Yutong Wang; Xuelian Xin; Huan Lin; Liangliang Zhang; Rongming Wang; Daofeng Sun

doi:10.1039/C7CC02134H

A non-interpenetrating lead-organic framework with large channels based on 1D tube-shaped SBUs†

Fangna Dai,

*^a Weidong Fan,^a Xue Yuan,^a Zhaodi Huang,^a Yutong Wang,

^a Xuelian Xin,^a Huan Lin,^a Liangliang Zhang,^a Rongming Wang^a and Daofeng Sun

*^a

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* Corresponding authors

^a State Key Laboratory of Heavy Oil Processing, College of Science, China University of Petroleum (East China), Qingdao Shandong 266580, People's Republic of China
E-mail: fndai@upc.edu.cn, dfsun@upc.edu.cn

Abstract

This work presents the construction of a porous lead-organic framework (UPC-10) with large channels of ∼24 Å. UPC-10 shows efficient adsorption of I₂ and selective adsorption of some dyes containing the SO₃⁻ group. After the adsorption of dyes, UPC-10 exhibits a CO₂ gas uptake ability. Furthermore, UPC-10 could be transformed into PbS in a H₂S atmosphere, and the derived PbS manifests N₂ and CO₂ uptake abilities.

Chemical Communications

A non-interpenetrating lead-organic framework with large channels based on 1D tube-shaped SBUs†

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A non-interpenetrating lead-organic framework with large channels based on 1D tube-shaped SBUs

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