Coupling between the photo-excited cyclic π system and the 4f electronic system in a lanthanide single molecule magnet

K. Kizaki; H. Ozawa; T. Kobayashi; R. Matsuoka; Y. Sakaguchi; A. Fuyuhiro; T. Fukuda; N. Ishikawa

doi:10.1039/C7CC02960H

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Coupling between the photo-excited cyclic π system and the 4f electronic system in a lanthanide single molecule magnet†

K. Kizaki,^a H. Ozawa,^a T. Kobayashi,^a R. Matsuoka,‡^a Y. Sakaguchi,^a A. Fuyuhiro,^a T. Fukuda^a and N. Ishikawa

*^a

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* Corresponding authors

^a Department of Chemistry, Graduate School of Science, Osaka University, Machikaneyamacho, Toyonaka, Osaka 560-0043, Japan
E-mail: iskw@chem.sci.osaka-u.ac.jp

Abstract

A new type of electronic interaction which couples two angular momenta, i.e. the angular momentum of a localized 4f system (J) and an orbital angular momentum generated in a cyclic π conjugated system by irradiation with a circularly-polarized light, has been identified in a lanthanide single molecule magnet.

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Article information

DOI: https://doi.org/10.1039/C7CC02960H
Article type: Communication
Submitted: 18 Apr 2017
Accepted: 12 May 2017
First published: 23 May 2017

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Chem. Commun., 2017,53, 6168-6171

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Coupling between the photo-excited cyclic π system and the 4f electronic system in a lanthanide single molecule magnet

K. Kizaki, H. Ozawa, T. Kobayashi, R. Matsuoka, Y. Sakaguchi, A. Fuyuhiro, T. Fukuda and N. Ishikawa, Chem. Commun., 2017, 53, 6168 DOI: 10.1039/C7CC02960H

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Chemical Communications

Coupling between the photo-excited cyclic π system and the 4f electronic system in a lanthanide single molecule magnet†

Abstract

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Coupling between the photo-excited cyclic π system and the 4f electronic system in a lanthanide single molecule magnet

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