Metal-free redox active deep eutectic solvents†
J. C.
Goeltz 
*a
and
L. N.
Matsushima
a
*a
and
L. N.
Matsushima
a
Abstract
Metal-free deep eutectic solvents composed of hydrogen bond donors and viologen-based ammonium salts exhibit reversible electrochemistry with viologen concentrations of 4.2 M and freezing points near room temperature. Spectroelectrochemistry and simulation of voltammetry indicate poor aggregation of the reduced radical cation.
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