A mesoinic pyridylideneamide ligand (PYA) was synthetized and fully characterized and coordinated to an iridium(III) center. This ligand represents the first example of a mesoionic N-donor ligand. Structural and spectroscopic analysis revealed unique properties which were exploited in chemically driven water oxidation catalysis.
M. Navarro, M. Li, S. Bernhard and M. Albrecht, Dalton Trans., 2018, 47, 659 DOI: 10.1039/C7DT04555G
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