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Abstract | Cited by

A scandium complex based on a new type of tridentate ligand enabled an atom- and step-economical C(sp3)–H addition of N,N-dimethyl anilines to a variety of unactivated alkenes affording branched products for the first time. A cationic o-dimethylaminophenyl scandium species was isolated and confirmed as the catalytic intermediate in this transformation.

Graphical abstract: Scandium-catalyzed C(sp3)–H alkylation of N,N-dimethyl anilines with alkenes

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