Ultrahigh-performance tungsten-doped perovskites for the oxygen evolution reaction

Gao Chen; Zhiwei Hu; Yanping Zhu; Zhi-Gang Chen; Yijun Zhong; Hong-Ji Lin; Chien-Te Chen; Liu Hao Tjeng; Wei Zhou; Zongping Shao

doi:10.1039/C8TA02864H

Ultrahigh-performance tungsten-doped perovskites for the oxygen evolution reaction†

Gao Chen,^a Zhiwei Hu,^b Yanping Zhu,^a Zhi-Gang Chen,^c Yijun Zhong,

^d Hong-Ji Lin,^e Chien-Te Chen,^e Liu Hao Tjeng,^b Wei Zhou

*^a and Zongping Shao

*^ad

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* Corresponding authors

^a Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, No. 5 Xin Mofan Road, Nanjing 210009, P. R. China
E-mail: zhouwei1982@njtech.edu.cn, shaozp@njtech.edu.cn

^b Max-Planck-Institute for Chemical Physics of Solids, Nöthnitzer Street 40, Dresden 01187, Germany

^c Centre for Future Materials, University of Southern Queensland, Springfield, Queensland 4300, Australia

^d Department of Chemical Engineering, Curtin University Perth, Western Australia 6845, Australia

^e National Synchrotron Radiation Research Center, 101 Hsin-Ann Road, Hsinchu 30076, Taiwan, Republic of China

Abstract

Here, using the materials genome strategy, we can account for the comprehensive effects of composition, structure, active sites and adsorption energy, and identify a novel B-site cation ordered double perovskite, SrCo_0.4Fe_0.2W_0.4O_3−δ (SCFW_0.4), as a superior OER electrocatalyst, which shows outstanding activity and excellent operational stability.

Journal of Materials Chemistry A

Ultrahigh-performance tungsten-doped perovskites for the oxygen evolution reaction†

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Ultrahigh-performance tungsten-doped perovskites for the oxygen evolution reaction

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