De novo synthesis of Cr-embedded MOF-199 and derived porous CuO/CuCr2O4 composites for enhanced phenol hydroxylation

Yu-Yuan Huang; Hannelore Konnerth; Jyun-Yi Yeh; Martin H. G. Prechtl; Cheng-Yen Wen; Kevin C.-W. Wu

doi:10.1039/C8GC03348J

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De novo synthesis of Cr-embedded MOF-199 and derived porous CuO/CuCr₂O₄ composites for enhanced phenol hydroxylation†

Yu-Yuan Huang,^a Hannelore Konnerth,^ab Jyun-Yi Yeh,^a Martin H. G. Prechtl,

^bf Cheng-Yen Wen

^cde and Kevin C.-W. Wu

*^ade

Author affiliations

* Corresponding authors

^a Department of Chemical Engineering, National Taiwan University (NTU), No. 1, Sec. 4, Roosevelt Road, Taipei 10617, Taiwan
E-mail: kevinwu@ntu.edu.tw

^b Department of Chemistry, Institute of Inorganic Chemistry, University of Cologne, Greinstr. 6, 50939 Cologne, Germany

^c Department of Materials Science and Engineering, National Taiwan University, Taiwan

^d Center of Atomic Initiative for New Materials (AI-MAT), NTU, Taiwan

^e International Graduate Program of Molecular Science and Technology, National Taiwan University (NTU-MST), Taiwan

^f Department of Natural Science and Environment, Roskilde University, Universitetsvej 1, 4000 Roskilde, Denmark

Abstract

A de novo synthesis of Cr-embedded MOF-199 was developed for the first time. This Cr-MOF-199 material was further derived into CuO/CuCr₂O₄ composites with a porous and uniform structure. The obtained bimetallic oxides with a porous structure were further applied in phenol hydroxylation.

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Article information

DOI: https://doi.org/10.1039/C8GC03348J
Article type: Communication
Submitted: 25 Oct 2018
Accepted: 04 Feb 2019
First published: 07 Feb 2019

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Green Chem., 2019,21, 1889-1894

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De novo synthesis of Cr-embedded MOF-199 and derived porous CuO/CuCr₂O₄ composites for enhanced phenol hydroxylation

Y. Huang, H. Konnerth, J. Yeh, M. H. G. Prechtl, C. Wen and K. C.-W. Wu, Green Chem., 2019, 21, 1889 DOI: 10.1039/C8GC03348J

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