Issue 50, 2019, Issue in Progress
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RSC Advances

One-step solution synthesis of a two-dimensional semiconducting covalent organometallic nanosheet via the condensation of boronic acid†

Qijun Wang,‡a   Jiahao Yan,‡b   Mingchao Xiao,‡ac   Devaraj Manoj,‡a   Cheng Zhong,e   Qiying Lv, ORCID logo a   Lite Yang,a   Liangmei Wu,b   Zhuoping Wang,a   Lihong Bao, ORCID logo *b   Hongjun Gao, ORCID logo b   Fei Xiao,a   Lang Jiang ORCID logo c  and  Shuai Wang ORCID logo *ad  

* Corresponding authors

a School of Chemistry and Chemical Engineering, Huazhong University of Science & Technology, Wuhan, P. R. China
E-mail: chmsamuel@mail.hust.edu.cn

b Institute of Physics, Chinese Academy of Sciences, Beijing 100190, P. R. China
E-mail: lhbao@iphy.ac.cn

c Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, P. R. China

d Department of Materials Science, Fudan University, Shanghai, P. R. China

e College of Chemistry and Molecular Sciences, Wuhan University, Wuhan, P. R. China

Abstract

In this work, a 2D covalent organometallic nanosheet (COMS) was designed and successfully synthesized through the one-step conjunction of a terpyridine–metal–terpyridine (TMT) sandwich coordinate motif with borate ester covalent heterocyclic (B3O3) linkage via the condensation of boronic acid. The obtained 2D COMS with a cobalt coordination center (2D COMS-Co) showed promising p-type semiconducting properties.

Graphical abstract: One-step solution synthesis of a two-dimensional semiconducting covalent organometallic nanosheet via the condensation of boronic acid

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Article information

DOI
https://doi.org/10.1039/C9RA05806K
Article type
Paper
Submitted
26 Jul 2019
Accepted
02 Sep 2019
First published
17 Sep 2019
This article is Open Access
Creative Commons BY-NC license

RSC Adv., 2019,9, 29327-29330

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One-step solution synthesis of a two-dimensional semiconducting covalent organometallic nanosheet via the condensation of boronic acid

Q. Wang, J. Yan, M. Xiao, D. Manoj, C. Zhong, Q. Lv, L. Yang, L. Wu, Z. Wang, L. Bao, H. Gao, F. Xiao, L. Jiang and S. Wang, RSC Adv., 2019, 9, 29327 DOI: 10.1039/C9RA05806K

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