The first example of diamino-benzoquinonediimine bearing both electron-donating and electron-withdrawing groups on the same 6-π electron subunit was synthesized using a straightforward one pot strategy. Photophysical analysis and theoretical calculations demonstrate that this unique substitution pattern is efficient to favour the establishment of a single tautomeric structure in solution.
J. Longevial, Z. Chen, S. Pascal, G. Canard, D. Jacquemin and O. Siri, Chem. Commun., 2021, 57, 548 DOI: 10.1039/D0CC06815B
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