On-demand hydrogen release could be an important process for the transportation of fuel in the near future. Herein it is reported that the controlled thermolysis of HKUST-1 under optimal conditions generates structural defects resulting in a quasi-HKUST-1 material showing a 20-fold enhancement of the H2 release turnover frequency at room temperature in the absence of a base.
M. Bagheri, A. Melillo, B. Ferrer, M. Y. Masoomi and H. Garcia, Chem. Commun., 2021, 57, 11964 DOI: 10.1039/D1CC05182B
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