Issue 55, 2024

Energy level regulation of anions via hydrogen bond effects to construct a stable solid electrolyte interface for a high-stability lithium metal anode

Abstract

An intermolecular hydrogen bond between 2,5-dihydroxyterephthalic acid and the anions in the Li+ solvation shell is constructed to promote the formation of a LiF-rich SEI on a metallic Li electrode. Li metal batteries with improved cyclability (140 cycles under an N/P ratio of 4.9) and high capacity retention (90%) are eventually obtained.

Graphical abstract: Energy level regulation of anions via hydrogen bond effects to construct a stable solid electrolyte interface for a high-stability lithium metal anode

Supplementary files

Article information

Article type
Communication
Submitted
06 May 2024
Accepted
12 Jun 2024
First published
19 Jun 2024

Chem. Commun., 2024,60, 7045-7048

Energy level regulation of anions via hydrogen bond effects to construct a stable solid electrolyte interface for a high-stability lithium metal anode

C. Wang, S. Liu, X. Wang, G. Tian, F. Fan, P. Liu, S. Wang, C. Zeng and C. Shu, Chem. Commun., 2024, 60, 7045 DOI: 10.1039/D4CC01981D

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