Versatile cross-dehydrogenative coupling of heteroaromatics and hydrogen donors via decatungstate photocatalysis

Matteo C. Quattrini; Saki Fujii; Keiichi Yamada; Takahide Fukuyama; Davide Ravelli; Maurizio Fagnoni; Ilhyong Ryu

doi:10.1039/C6CC09725A

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Versatile cross-dehydrogenative coupling of heteroaromatics and hydrogen donors via decatungstate photocatalysis†

Matteo C. Quattrini,^a Saki Fujii,^b Keiichi Yamada,^b Takahide Fukuyama,^b Davide Ravelli,

*^a Maurizio Fagnoni^a and Ilhyong Ryu*^bc

Author affiliations

* Corresponding authors

^a PhotoGreen Lab, Department of Chemistry, University of Pavia, Viale Taramelli 12, 27100 Pavia, Italy
E-mail: davide.ravelli@unipv.it

^b Department of Chemistry, Graduate School of Science, Osaka Prefecture University, Sakai, Osaka 599-8531, Japan
E-mail: ryu@c.s.osakafu-u.ac.jp

^c Department of Applied Chemistry, National Chiao Tung University, Hsinchu, Taiwan

Abstract

A facile sunlight-induced derivatization of heteroaromatics via photocatalyzed C–H functionalization in amides, ethers, alkanes and aldehydes is described. Tetrabutylammonium decatungstate (TBADT) was used as the photocatalyst and allowed to carry out the process under mild conditions.

This article is part of the themed collection: Site-selective molecular transformations

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Article information

DOI: https://doi.org/10.1039/C6CC09725A
Article type: Communication
Submitted: 07 Dec 2016
Accepted: 25 Jan 2017
First published: 25 Jan 2017

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Chem. Commun., 2017,53, 2335-2338

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Versatile cross-dehydrogenative coupling of heteroaromatics and hydrogen donors via decatungstate photocatalysis

M. C. Quattrini, S. Fujii, K. Yamada, T. Fukuyama, D. Ravelli, M. Fagnoni and I. Ryu, Chem. Commun., 2017, 53, 2335 DOI: 10.1039/C6CC09725A

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Chemical Communications

Versatile cross-dehydrogenative coupling of heteroaromatics and hydrogen donors via decatungstate photocatalysis†

Abstract

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Versatile cross-dehydrogenative coupling of heteroaromatics and hydrogen donors via decatungstate photocatalysis

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