Construction of robust Cu-MOFs from bifunctional pyridine-hydroxamate linkers for photocatalytic CO2 reduction

Li Xiong; Wenlei Tang; Chaozhi Xiong; Jiajun Du; Zhiyuan Zhang; Yuqing Qiu; Zhen-Wu Shao; Xuemei Zhou; Chong Liu

doi:10.1039/D4CC06778A

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Construction of robust Cu-MOFs from bifunctional pyridine-hydroxamate linkers for photocatalytic CO₂ reduction†

Li Xiong,^a Wenlei Tang,^a Chaozhi Xiong,^a Jiajun Du,^a Zhiyuan Zhang,^a Yuqing Qiu,^a Zhen-Wu Shao,

*^a Xuemei Zhou

*^a and Chong Liu

*^a

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* Corresponding authors

^a School of Chemical Engineering, Sichuan University, Chengdu, China
E-mail: liuchong@scu.edu.cn, xuemeizhou@scu.edu.cn, 2021323070018@stu.scu.edu.cn

Abstract

Robust Cu-MOFs with distinct topologies were prepared from the same bifunctional 4-pyridine-hydroxamate ligand. A favourable collection of porosity, framework stability, electronic structure, and photochemical properties was revealed for the SUM-33 MOF, which was later experimentally verified as an efficient and selective photocatalyst for CO₂-to-CO conversion.

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DOI: https://doi.org/10.1039/D4CC06778A
Article type: Communication
Submitted: 29 Dec 2024
Accepted: 07 Feb 2025
First published: 10 Feb 2025

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Chem. Commun., 2025, Advance Article

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Construction of robust Cu-MOFs from bifunctional pyridine-hydroxamate linkers for photocatalytic CO₂ reduction

L. Xiong, W. Tang, C. Xiong, J. Du, Z. Zhang, Y. Qiu, Z. Shao, X. Zhou and C. Liu, Chem. Commun., 2025, Advance Article , DOI: 10.1039/D4CC06778A

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