Enhanced carrier transport of monolayer MoSe2 through interlayer coupling with in situ grown metal–organic frameworks

Abstract

Exceptional interlayer coupling of organic–inorganic vdWHs is paramount for enhancing electron mobility. Herein, we report a novel transfer-free method to fabricate MoSe₂/Ni₃(HITP)₂ vdWHs. The MOF film promotes interfacial charge transfer, leading to a threefold increase in electron mobility. This work provides a platform for developing high-performance optoelectronic devices.