‘Vitrimer nanocomposites’ derived from graphene oxide and post-consumer recycled polypropylene

Abstract

Post-consumer recycled polypropylene (PCR PP) is promising for sustainable applications, yet its limitations in electrical conductivity and mechanical properties require modifications. This study develops a vitrimer nanocomposite by modifying PCR PP via styrene-assisted maleic anhydride grafting and incorporating a molecule containing multiple epoxide groups facilitating effective crosslinking. Graphene oxide (GO) is added as a nanofiller, improving rheological, thermal, electrical and infrared thermal properties. Characterization techniques confirm structural enhancements, while tensile testing shows significant gains in strength and modulus. The vitrimer nanocomposite demonstrates recyclability and high performance, offering a sustainable path for advanced engineering applications within a circular economy framework.