Simple, easily available diamidocarbazoles 1–4 form robust 2 : 1 complexes with SO42− even in the presence of a large excess of water. An appropriate choice of side arms directs the assembly towards the formation of either an orthogonal or a biplane structure, both in solution and in the solid state.
K. M. Bąk and M. J. Chmielewski, Chem. Commun., 2014, 50, 1305 DOI: 10.1039/C3CC48463G
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