Efficient asymmetric bio-epoxidation of electron-deficient α,β-unsaturated ketones was realized via a tandem reduction-epoxidation-dehydrogenation cascade, which proceeds in a switchable manner to afford either chiral epoxy ketones or allylic epoxy alcohols with up to >99% yield and >99%ee.
Y. Liu and Z. Wu, Chem. Commun., 2016, 52, 1158 DOI: 10.1039/C5CC07548C
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